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In-situ electronic characterization of graphene nanoconstrictions fabricated in a transmission electron microscope

机译:石墨烯纳米限制的原位电子表征   在透射电子显微镜中制造

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摘要

We report electronic measurements on high-quality graphene nanoconstrictions(GNCs) fabricated in a transmission electron microscope (TEM), and the firstmeasurements on GNC conductance with an accurate measurement of constrictionwidth down to 1 nm. To create the GNCs, freely-suspended graphene ribbons werefabricated using few-layer graphene grown by chemical vapor deposition. Theribbons were loaded into the TEM, and a current-annealing procedure was used toclean the material and improve its electronic characteristics. The TEM beam wasthen used to sculpt GNCs to a series of desired widths in the range 1 - 700 nm;after each sculpting step, the sample was imaged by TEM and its electronicproperties measured in-situ. GNC conductance was found to be remarkably high,comparable to that of exfoliated graphene samples of similar size. The GNCconductance varied with width approximately as, where w is the constrictionwidth in nanometers. GNCs support current densities greater than 120 \muA/nm2,two orders of magnitude higher than has been previously reported for graphenenanoribbons and 2000 times higher than copper.
机译:我们报告了在透射电子显微镜(TEM)中制造的高质量石墨烯纳米缩颈(GNC)的电子测量结果,以及精确测量缩颈宽度低至1 nm的GNC电导率的首次测量结果。为了创建GNC,使用通过化学气相沉积法生长的几层石墨烯来制造自由悬浮的石墨烯带。将碳带加载到TEM中,并使用电流退火程序清洁该材料并改善其电子特性。然后使用TEM光束将GNC雕刻为一系列所需宽度,范围为1-700 nm;在每个雕刻步骤之后,通过TEM对样品进行成像,并就地测量其电子性能。发现GNC电导率非常高,与相似大小的脱落石墨烯样品的电导率相当。 GNC电导随宽度变化大约为,其中w是收缩宽度(以纳米为单位)。 GNC支持的电流密度大于120μA/ nm2,比以前报道的石墨烯纳米管高两个数量级,比铜高2000倍。

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